Værløse was a municipality (Danish, kommune) consisting of only one parish also named Værløse in the former Copenhagen County on the island of Zealand (Sjælland) in eastern Denmark. The municipality covered an area of 34 km², and in 2005 had a total population of 18,649. Its last mayor was Jesper Bach, a member of the Venstre (Liberal Party) political party. He was the first mayor of the newly formed Furesø municipality. The community is connected by a road and a motorway and commuter railway to Farum to the north via an isthmus at Fiskebæk between Lake Farum sø and Lake Furesø. The road and motorway run through a small forest on the western shore of Lake Furesø and is almost out of sight and hearing distance from nearby homes in Værløse, but north of the isthmus they run through the town of Farum, separating it in a western and eastern part.
The main town and the site of its municipal council was the town of Værløse. Other towns in the former municipality are Hareskovby, Kirke Værløse, and Jonstrup.
Neighboring municipalities were Farum to the north, Stenløse to the west, Ballerup and Herlev to the south, and Gladsaxe, Lyngby-Taarbæk and Søllerød to the east, albeit the last of these is separated physically from the municipality by the waters of Lake Furesø.