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The Japanese animated television series Last Exile has a cast of characters designed by artist Range Murata.

All names are displayed according to their spelling in the English subtitled version of the series, as released by Funimation Entertainment or in the romanization of the Japanese names as they appear on official merchandise published after the English localization of the series.

The initial concept designs for Last Exile were created by character designer Range Murata. Murata also spent a great amount of time on costume design. Wanting to portray each character's personality more fully, he "tried to draw in the kind of material that would have been used in creating their clothes and try to represent the stitches connecting the fabric". Although Gonzo initially intended for Last Exile to be shown in a space setting, it did not want characters who use sterile space suits. As a result, Murata's designs placed the show in its current setting.

Although the fictional world of Prester is not a representation of Earth, it features technology reminiscent of nineteenth century Europe at the dawn of the Industrial Revolution. Many of its designs were also inspired by Germany's technological advances during the interwar period. Uniform designs for Anatoray's musketeers were based on Napoleon Bonaparte's army and American Civil War soldiers. On the other hand, Soviet Red Army fur coats provided the basis for Disith uniforms. The crew of the Silvana wore uniforms that were more modern and utilitarian.

Production of Last Exile relied heavily on 3D computer animation. The animation for Last Exile was also supplemented with Victorian era flourishes. In order to combine hand-drawn animation with computer-generated ones, the production team used a technique for non-photorealistic rendering, which could not be used for Blue Submarine No. 6 (a previous work of Gonzo and one of the first CG anime series) because of a stylistic conflict. At the 2003 Anime Expo, production designer Mahiro Maeda, who also worked with Studio Ghibli's production of Laputa: Castle in the Sky, commented that "[Last Exile] is very advanced in how it will incorporate the two mediums".

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