"I'll Try Anything" was co-written by Mark Barkan and Vic [aka Victor] Millrose: Barkan had written the hits "I'm Gonna Be Warm This Winter" for Connie Francis and "I Don't Wanna Be a Loser" for Lesley Gore, while Millrose had written the Gene Pitney hit "Last Chance to Turn Around" and would later write "This Girl Is a Woman Now" for Gary Puckett & the Union Gap. Barkan, intending to write a song for Dusty Springfield, had already written the chorus for "I'll Try Anything" when Millrose came on board to co-write the verses. Springfield visited Barkan's residence to hear the song which Barkan sang to her while playing the piano, and although Springfield reacted favorably to the song she still wanted to hear a demo, and Barkan obliged by prepping a demo with Ellie Greenwich as vocalist.

Springfield began recording "I'll Try Anything" in a December 1966 session at the CBS Recording Studios (NYC) produced by Herb Bernstein: Barkan, who was present, recalls that the session lasted for nine hours with the first eight spent on Springfield recording another song: "The Morning After the Night Before", and the last hour spent on her recording "I'll Try Anything". On 22 January 1967 Springfield and Bernstein had another session at CBS Recording Studios which yielded a completed master of "I'll Try Anything": however Springfield elected to have the master's rhythm track extracted and used as the basis for a new recording of the song made at the Philips Studios in Stanhope Place in a 29 January 1967 session.

Since making her solo debut in 1963 with the upbeat "I Only Want to Be With You" Springfield had subsequently shifted her musical focus to a softer sound as exemplified by her 1966 career record "You Don't Have to Say You Love Me". "I'll Try Anything" was largely a return to Springfield's original upbeat sound and might have been a more substantial hit for her somewhat earlier. However, by 1967 the track had a markedly out-of-date sound and in its UK release peaked at #13 breaking a Top Ten streak for Springfield which had lasted for three hits.

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